Chip-based spectroscopy using microresonator frequency combs

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Abstract
The development of a spectroscopy device on a chip that could realize real-time, label-free and high-throughput detection of trace molecules presents one of the biggest challenges in sensing. This is particularly challenging in the mid-infrared (mid-IR) domain where strong and characteristic molecular absorption occurs but optical sources are still in full development. In the past decade, there has been a remarkable development of a miniaturized optical frequency comb source using parametric nonlinear interactions in microresonators. Such integrated devices present as unique tools for direct generation of broadband mid-IR light and ultrafast acquisition speed of molecular absorption information. In this thesis, we address the microresonator technology for the generation of a broadband modelocked frequency comb in the mid-IR. The properties of such microcombs can be precisely controlled, tuned, and characterized. We show that microresonator-based combs is not only an ideal testbed for studying a variety of nonlinear dynamics but, more importantly, can be used to realize a silicon-based platform for vibrational spectroscopy. We demonstrate two different types of mid-IR microcomb-based spectroscopy, dual-comb spectroscopy, and scanning comb spectroscopy which are suitable for condensed phase study and trace gas sensing, respectively.
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2018-08-30
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Applied physics; integrated optics; mid-infrared optics; nonlinear photonics; optical frequency combs; Infrared Spectroscopy; Silicon Photonics; Optics
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Lipson, Michal
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Rana, Farhan
Gaeta, Alexander L.
Degree Discipline
Electrical and Computer Engineering
Degree Name
Ph. D., Electrical and Computer Engineering
Degree Level
Doctor of Philosophy
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Government Document
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Attribution 4.0 International
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dissertation or thesis
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