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  4. A 10-fs Multicolor Source for Ultrafast Spectroscopy and Quantum Communication

A 10-fs Multicolor Source for Ultrafast Spectroscopy and Quantum Communication

File(s)
Heberle_cornellgrad_0058F_12890.pdf (15.28 MB)
Permanent Link(s)
https://doi.org/10.7298/j72j-tj57
https://hdl.handle.net/1813/110872
Collections
Cornell Theses and Dissertations
Author
Heberle, Dylan Andrew
Abstract

Broadband multicolor lasers are able to provide valuable information concerning ultrafast molecular dynamics through time-resolved spectroscopy. Here, I present my work developing a multicolor, 10-fs laser source through the marriage of three key technologies: (1) a high-repetition-rate, 10-fs, energetic NIR front end, (2) NIR pulse shaping, and (3) adiabatic frequency conversion. These technologies provide the means to generate femtosecond pulses in the visible, near-IR, and mid-IR with amplitude and phase control without multiple com plex dispersion-management schemes, constituting a toolbox of femtosecond pulses that can be used to probe fleeting molecular dynamics. 100-µJ, 10-fs pulses are generated from the NIR front end, which are shaped and compressed with NIR 4f pulse shapers and subsequently converted to 10-fs visible (MIR) pulse using dispersion-managed adiabatic sum (difference) frequency generation. Compression of the NIR pulses has been confirmed using SHG FROG. The MIR pulses were measured using a sensitive, phase-matching-free technique called frequency-resolved optical switching. Additionally, various ap plications are reviewed including quantum frequency homogenization, simultaneously converting visible single photons to the telecom C-band and reducing their spectral distinguishability, and ultrafast time-resolved spectroscopy experiments planned for single-layer graphene, rhodopsin and various mutants, and DNA.

Description
156 pages
Date Issued
2021-12
Keywords
adiabatic frequency conversion
•
multicolor femtosecond laser
•
nonlinear optics
•
quantum frequency conversion
•
ultrafast dynamics
Committee Chair
Moses, Jeffrey
Committee Member
Nishimura, Nozomi
Wise, Frank
Degree Discipline
Applied Physics
Degree Name
Ph. D., Applied Physics
Degree Level
Doctor of Philosophy
Type
dissertation or thesis
Link(s) to Catalog Record
https://newcatalog.library.cornell.edu/catalog/15312732

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