Mesoporous amine-bridged polysilsesquioxane for CO2 capture

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https://hdl.handle.net/1813/30468
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Author
Qi, G.; Fu, L.; Duan, X.; Choi, B-H.; Abraham, M.; Giannelis, E.P.
Abstract
A novel class of amine-supported sorbents based on amine-bridged mesoporous polysilsesquioxane was developed via a simple one-pot sol-gel process. The new sorbent allows the incorporation of a large amount of active groups without sacrificing surface area or pore volume available for CO2 capture, leading to a CO2 capture capacity of 3.2 mmol g−1 under simulated flue gas conditions. The sorbent is readily regenerated at 100°C and exhibits good stability over repetitive adsorption-desorption cycling. © 2011 Society of Chemical Industry and John Wiley & Sons, Ltd
Sponsorship
Th is publication was based on work supported by Award No. KUS-C1-018-02, made by King Abdullah University of Science and Technology (KAUST). Experimental details of the synthesis and characterization of the sorbent. Adsorption and desorption of the sorbent.
Date Issued
2011-08-04
Publisher
Society of Chemical Industry and John Wiley & Sons, Ltd
Subject
carbon dioxide capture; mesoporous; polysilsesquioxane; post-combustion
Related Version
http://onlinelibrary.wiley.com/doi/10.1002/ghg.26/abstract
Previously Published As
Greenhouse Gas Sci Technol. 1:278–284 (2011); DOI: 10.1002/ghg
Type
article

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