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  4. An Experimental Perspective on Exciton-Polariton Bose-Einstein Condensation

An Experimental Perspective on Exciton-Polariton Bose-Einstein Condensation

File(s)
Khazanov_cornellgrad_0058F_14922.pdf (26.5 MB)
No Access Until
2026-06-02
Permanent Link(s)
https://doi.org/10.7298/51kp-tv39
https://hdl.handle.net/1813/117584
Collections
Cornell Theses and Dissertations
Author
Khazanov, Thomas
Abstract

In this dissertation, we describe our investigation into exciton-polariton Bose-Einstein condensation in organic materials. Exciton-polaritons are hybrid quasiparticles arising from the interaction of an exciton with the electromagnetic field. As bosons, they undergo Bose-Einstein condensation at a critical density. In the first part of this work, we address the question of whether polariton condensates in organic materials can be considered true Bose-Einstein condensates. We build on this work to investigate the mechanism of condensation in the semiconducting polymer poly(9,9-di-n-octylfluorenyl-2,7-diyl). Finally, we consider reports of enhanced internal conversion rates in zinc tetraphenylporphyrin through strong light-matter coupling and attempt to ascertain the origin of this effect and its implications for condensation and polariton chemistry.

Description
143 pages
Date Issued
2025-05
Keywords
Bose-Einstein condensation
•
exciton
•
polariton
•
quantum optics
•
ultrafast spectroscopy
Committee Chair
Musser, Andrew
Committee Member
Marohn, John
Ananth, Nandini
Degree Discipline
Chemistry and Chemical Biology
Degree Name
Ph. D., Chemistry and Chemical Biology
Degree Level
Doctor of Philosophy
Rights
Attribution 4.0 International
Rights URI
https://creativecommons.org/licenses/by/4.0/
Type
dissertation or thesis
Link(s) to Catalog Record
https://newcatalog.library.cornell.edu/catalog/16938200

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